What do you think of the games you haven't played before?
I think Balloon Fight is a lot of fun, and Wrecking Crew is also pretty good. Ice Climber is okay, but the jumping is pretty sloppy. D.K. Jr. is ruined with terrible jumping. Yoshi is just boring. NES Open Tournament Golf is pretty deep for an NES sports game, but the super fast meter return makes it extremely hard to hit the ball with any kind of accuracy. Zelda will probably be more interesting once I get going, but so far I can't find anything to do except fight enemies for rupees until I have enough to buy something in one of the two shops I've found. I haven't tried Zelda II yet.
I've already got Super Mario Bros. and Metroid on the Wii's VC, so I already know what to expect with those.